团队介绍
“电子与光学课题组(The Electronics & Optics Group)“致力于通过调控半导体中电子行为及其光学响应,完成高效可控的化学反应,以解决国家“双碳“战略需求相关问题。近五年,为实现光催化中增加光子吸收、促进电荷转移、控制表面反应等目标,从材料、机理、反应等角度开展了以下工作。1. 探明聚合物连接体与电子能带之间关系,开发带隙连续可调的新型光催化剂,全可见光下高效制氢。2. 搭建微秒瞬态吸收光谱,阐明碳点结构与其光物理性质关系,实现近100%选择性的CO2 制甲醇(第26届联合国气候变化缔约方大会COP26收录)。3. 开发了无需搅拌的多层光反应器件,实现了低能垒的碱性甲醇重整高效制氢。
PI近五年在国际期刊发表SCI论文15篇,其中以第一作者在Nat. Energy, Nat. Commun., Angew. Chem., EES等期刊发表论文10篇,ESI高引4篇,总引1900余次,h因子为12。为Frontiers 系列期刊客座编辑, 十余国际期刊审稿人,德国洪堡学者,英国皇家化学会会员。
欢迎各位对物理化学感兴趣的同学来我们课题组开展研究或攻读学位,也欢迎各位同行交流合作。
论文
(1) Yiou Wang; Anastasia Vogel; Michael Sachs; Reiner Sebastian Sprick; Liam Wilbraham; Savio J. A. Moniz; Robert Godin; Martijn A. Zwijnenburg; James R. Durrant; Andrew I. Cooper; Junwang Tang ; Current understanding and challenges of solar-driven hydrogen generation using polymeric photocatalysts, Nature Energy, 2019, 4: 746-760.
(2) Yiou Wang; Xu Liu; Xiaoyu Han; Robert Godin; Jialu Chen; Wuzong Zhou; Chaoran Jiang; Jamie F. Thompson; Bayazit K. Mustafa; Stephen A. Shevlin; James R. Durrant; Zhengxiao Guo; Junwang Tang ; Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water, Nature Communications, 2020, 11,2531.
(3) Yiou Wang; Robert Godin; James R Durrant; Junwang Tang ; Efficient Hole Trapping in Carbon Dot/Oxygen-Modified Carbon Nitride Heterojunction Photocatalysts for Enhanced Methanol Production from CO2 under Neutral Conditions, Angewandte Chemie International Edition, 2021, 60: 20811-20816.
(4) Yiou Wang; En-Ping Yao; Linzhong Wu; Jochen Feldmann.; Jacek K. Stolarczyk ; A Multi-Layer Device for Light-Triggered Hydrogen Production from Alkaline Methanol, Angewandte Chemie International Edition, 2021, 60: 26694-26701.
(5) Yiou Wang; Mustafa K. Bayazit; Savio J. A. Moniz; Qiushi Ruan; Chi Ching Lau; Natalia Martsinovich; Junwang Tang ; Linker-controlled polymeric photocatalyst for highly efficient hydrogen evolution from water, Energy & Environmental Science, 2017, 10: 1643-1651.
(6) Yiou Wang; Enqi Chen; Junwang Tang; Insight on Reaction Pathways of Photocatalytic CO2 Conversion, ACS Catalysis, 2022, doi.org/10.1021/acscatal.2c01012.
(7) Linzhong Wu; Yiou Wang; Mariam Kurashvili; Amrita Dey; Muhan Cao; Markus D?blinger; Qiao Zhang; Jochen Feldmann; He Huang; Tushar Debnath ; Interfacial Manganese-Doping in CsPbBr3 Nanoplatelets by Employing a Molecular Shuttle, Angewandte Chemie International Edition, 2022, 61, e202115852.
(8) Yiou Wang; Hajime Suzuki; Jijia Xie; Osamu Tomita; David James Martin; Masanobu Higashi; Dan Kong; Ryu Abe; Junwang Tang ; Mimicking Natural Photosynthesis: Solar to Renewable H2 Fuel Synthesis by Z-Scheme Water Splitting Systems, Chemical Reviews, 2018, 118(10): 5201-5241.
(9) Yiou Wang; Fabrizio Silveri; Mustafa K. Bayazit; Qiushi Ruan; Yaomin Li; Jijia Xie; C. Richard A. Catlow; Junwang Tang ; Bandgap Engineering of Organic Semiconductors for Highly Efficient Photocatalytic Water Splitting, Advanced Energy Materials, 2018, 8: 1801084.
(10) Robert Godin; Yiou Wang; Martijn A. Zwijnenburg; Junwang Tang; James R. Durrant ; Time-Resolved Spectroscopic Investigation of Charge Trapping in Carbon Nitrides Photocatalysts for Hydrogen Generation, Journal of the American Chemical Society, 2017, 139(14): 5216-5224.